The Cape of Good Hope tour is awesome, you will definately get some awesome shots there.
Cape Town isnt as bad as Johannesburg in terms of crime, although that doesnt mean you dont have to be vigiliant. You could maybe also enquire about boat trips from Houtbay to Seal island (would also make for some awesome shots and you may very well see a great white)
Then, if you havent been up Table mountain, do it, but go very early, trust me. The queues are ridiculous.
If you're renting a car, it may also be worth your while to go up to signal hill (heard it's dangerous there at night, I havent experienced it yet) But early morning and dawn should be fine. It'll allow you shots of the entire Cape Harbor, Cape Town, and coastline leading up to the westcoast.
From there, travel backwards toward Camps bay (very posh, trendy, but extremely beautiful beach) and travel over Sir Lowry's Pass further on to reach awesome little picturesque 'dorpies' along the way.
Hope this helps :)
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